Scarlett Johansson Natasha Romanoff / Black Widow
Samuel L. Jackson Nick Fury
Anthony Mackie Sam Wilson / Falcon
Elizabeth Olsen Wanda Maximoff / Scarlet Witch (uncredited)
Hayley Atwell Peggy Carter
Sebastian Stan Bucky Barnes / Winter Soldier
Cobie Smulders Maria Hill
Toby Jones Dr. Arnim Zola
Emily VanCamp Kate / Agent 13
Danny Pudi Com Tech #1
Chris Evans Steve Rogers / Captain America
Frank Grillo Brock Rumlow
Steve Constancio Costumer
Sarah Halley Finn Casting
Nestor Serrano Committee General (uncredited)
Robert Clotworthy Fury Car Voice (voice)
Robert Redford Alexander Pierce
Aaron Taylor-Johnson Pietro Maximoff / Quicksilver (uncredited)
Gary Sinise The Smithsonian Narrator (voice)
Stan Lee Smithsonian Guard, Executive Producer, Thanks
Jenny Agutter Councilwoman Hawley
Steven Culp Scudder
Randall L. Johnson Boom Operator
Clay Cullen Stunt Double
Jon H. Epstein Utility Stunts
Zack Duhame Engine Pirate, Stunts
Beat Frutiger Art Direction
Kevin Feige Producer
Wendy Hoopes Doctor
Pete Romano Underwater Director of Photography
Steve Upton Utility Stunts
Heba Thorisdottir Makeup Artist
Maryellen Aviano Extras Casting
Salvator Xuereb French Pirate #1
Louis D'Esposito Executive Producer
Jack Kirby Comic Book
Joss Whedon Man on Escalator in Museum (uncredited)
Casey O'Neill Stunt Coordinator
Anthony Russo Director
Steele Hunter Rigging Grip
Adetokumboh M'Cormack French Radio Pirate
Nancy Keslar Hairstylist
Thomas Nittmann Visual Effects Producer
Alan Dale Councilman Rockwell
John St. Laurent Dailies Operator
Greg Hale Second Assistant Director
Jeremy Fitzgerald Utility Stunts
Joe Russo Dr. Fine, Director
Thomas Kretschmann Baron Wolfgang von Strucker (uncredited)
Callan Mulvey Jack Rollins
Garry Shandling Senator Stern
Richard Crompton Rigging Grip
Amy Johnston Stunt Double
Don Heck Thanks
Victoria Alonso Executive Producer
Roger Wall Second Assistant "A" Camera
Paul Sonski Set Designer
Dominic Rains CIA Instructor
Joe Bucaro III Utility Stunts
Jack Glenn Dolly Grip
Holland Diaz Stunt Double
Henry Goodman Dr. List (uncredited)
Danny Rafic Visual Effects Editor
Ricardo Chacon Strike SGT. #1
Mark Santoni First Assistant "B" Camera
Eddie J. Fernandez Strike Agent
Pat Healy Scientist #1
Daniel Hargrave Stunt Double
Jon Sklaroff Charlie XO
James D. Wickman Dolly Grip
Dana Baker Best Boy Grip
Carrie Arakaki Costumer